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Article: One-Photon Upconversion-Like Photolysis: A New Strategy to Achieve Long-Wavelength Light-Excitable Photolysis

TitleOne-Photon Upconversion-Like Photolysis: A New Strategy to Achieve Long-Wavelength Light-Excitable Photolysis
Authors
KeywordsBODIPY
long-wavelength light excitation
photocleavable protecting groups
photocleavage
photon upconversion
Issue Date2020
PublisherThieme Publishing. The Journal's web site is located at http://www.thieme-chemistry.com/thieme-chemistry/journals/info/synlett/index.shtml
Citation
Synlett, 2020, v. 31 n. 12, p. 1129-1134 How to Cite?
AbstractPhotolysis reactions are widely utilized to release desired molecules under the control of light irradiation in the fields of photochemistry, biology, and drug delivery. In biological and medical applications, it is highly desired to increase the excitation wavelength for activating photolysis reactions, since the long-wavelength light (red or near-infrared light) has deep tissue penetration depth and low photocytotoxicity. Here, we briefly summarize current strategies of achieving long-wavelength light-excitable photolysis. We highlight our recently developed strategy of one-photon upconversion-like photolysis. Compared with the multiphoton upconversion-based photolysis, the one-photon strategy has a simpler energy transfer process and a higher energy utilization efficiency, providing a new path of activating photolysis reactions with increased excitation wavelength and photolysis quantum yield. © 2020 American Institute of Physics Inc.. All rights reserved.
Persistent Identifierhttp://hdl.handle.net/10722/290095
ISSN
2019 Impact Factor: 2.006
2015 SCImago Journal Rankings: 0.908

 

DC FieldValueLanguage
dc.contributor.authorLyu, W-
dc.contributor.authorWang, W-
dc.date.accessioned2020-10-22T08:22:02Z-
dc.date.available2020-10-22T08:22:02Z-
dc.date.issued2020-
dc.identifier.citationSynlett, 2020, v. 31 n. 12, p. 1129-1134-
dc.identifier.issn0936-5214-
dc.identifier.urihttp://hdl.handle.net/10722/290095-
dc.description.abstractPhotolysis reactions are widely utilized to release desired molecules under the control of light irradiation in the fields of photochemistry, biology, and drug delivery. In biological and medical applications, it is highly desired to increase the excitation wavelength for activating photolysis reactions, since the long-wavelength light (red or near-infrared light) has deep tissue penetration depth and low photocytotoxicity. Here, we briefly summarize current strategies of achieving long-wavelength light-excitable photolysis. We highlight our recently developed strategy of one-photon upconversion-like photolysis. Compared with the multiphoton upconversion-based photolysis, the one-photon strategy has a simpler energy transfer process and a higher energy utilization efficiency, providing a new path of activating photolysis reactions with increased excitation wavelength and photolysis quantum yield. © 2020 American Institute of Physics Inc.. All rights reserved.-
dc.languageeng-
dc.publisherThieme Publishing. The Journal's web site is located at http://www.thieme-chemistry.com/thieme-chemistry/journals/info/synlett/index.shtml-
dc.relation.ispartofSynlett-
dc.rightsSynlett. Copyright © Thieme Publishing.-
dc.subjectBODIPY-
dc.subjectlong-wavelength light excitation-
dc.subjectphotocleavable protecting groups-
dc.subjectphotocleavage-
dc.subjectphoton upconversion-
dc.titleOne-Photon Upconversion-Like Photolysis: A New Strategy to Achieve Long-Wavelength Light-Excitable Photolysis-
dc.typeArticle-
dc.identifier.emailLyu, W: lyuwen@hku.hk-
dc.identifier.emailWang, W: wangwp@hku.hk-
dc.identifier.authorityWang, W=rp02227-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1055/s-0040-1707100-
dc.identifier.scopuseid_2-s2.0-85087874032-
dc.identifier.hkuros315976-
dc.identifier.volume31-
dc.identifier.issue12-
dc.identifier.spage1129-
dc.identifier.epage1134-
dc.publisher.placeGermany-

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