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Article: The Molecule-Electrode Interface in Single-Molecule Transistors

TitleThe Molecule-Electrode Interface in Single-Molecule Transistors
Authors
Yu, HongbinLuo, YiBeverly, KristenStoddart, J. FraserTseng, Hsian RongHeath, James R.
KeywordsBreak junctions
Differential conductance
Molecular devices
Molecule electrode contact
Rotaxanes
Issue Date2003
Citation
Angewandte Chemie - International Edition, 2003, v. 42, n. 46, p. 5706-5711 How to Cite?
DOI: http://dx.doi.org/10.1002/anie.200352352
AbstractWhat's in the middle matters little! Differential conductance measurements made on single-molecule rotaxanes and their precursor dumbbells in transistors with platinum electrodes reflect the molecule-electrode contacts rather than the middle section of the molecules (see diagram; the color reflects the conductance, with dark corresponding to zero current). Interface states dominate electron transport. Molecular signatures are masked and even constitutional asymmetry in the molecule is difficult to detect.
Persistent Identifierhttp://hdl.handle.net/10722/332563
ISSN
1433-7851
2021 Impact Factor: 16.823
2020 SCImago Journal Rankings: 5.831

 

DC FieldValueLanguage
dc.contributor.authorYu, Hongbin-
dc.contributor.authorLuo, Yi-
dc.contributor.authorBeverly, Kristen-
dc.contributor.authorStoddart, J. Fraser-
dc.contributor.authorTseng, Hsian Rong-
dc.contributor.authorHeath, James R.-
dc.date.accessioned2023-10-06T05:12:30Z-
dc.date.available2023-10-06T05:12:30Z-
dc.date.issued2003-
dc.identifier.citationAngewandte Chemie - International Edition, 2003, v. 42, n. 46, p. 5706-5711-
dc.identifier.issn1433-7851-
dc.identifier.urihttp://hdl.handle.net/10722/332563-
dc.description.abstractWhat's in the middle matters little! Differential conductance measurements made on single-molecule rotaxanes and their precursor dumbbells in transistors with platinum electrodes reflect the molecule-electrode contacts rather than the middle section of the molecules (see diagram; the color reflects the conductance, with dark corresponding to zero current). Interface states dominate electron transport. Molecular signatures are masked and even constitutional asymmetry in the molecule is difficult to detect.-
dc.languageeng-
dc.relation.ispartofAngewandte Chemie - International Edition-
dc.subjectBreak junctions-
dc.subjectDifferential conductance-
dc.subjectMolecular devices-
dc.subjectMolecule electrode contact-
dc.subjectRotaxanes-
dc.titleThe Molecule-Electrode Interface in Single-Molecule Transistors-
dc.typeArticle-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1002/anie.200352352-
dc.identifier.scopuseid_2-s2.0-0347504886-
dc.identifier.volume42-
dc.identifier.issue46-
dc.identifier.spage5706-
dc.identifier.epage5711-

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