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Article: Synthetic Tailoring of Graphene Nanostructures with Zigzag‐Edged Topologies: Progress and Perspectives
Title | Synthetic Tailoring of Graphene Nanostructures with Zigzag‐Edged Topologies: Progress and Perspectives |
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Authors | |
Keywords | Bottom-up synthesis Doping Graphene nanoribbons Magnetism Nanographenes |
Issue Date | 2020 |
Publisher | Wiley - VCH Verlag GmbH & Co. KGaA. The Journal's web site is located at http://www3.interscience.wiley.com/journal/26737/home |
Citation | Angewandte Chemie (International Edition), 2020, v. 59 n. 52, p. 23386-23401 How to Cite? |
Abstract | Both experimental and theoretical investigations have revealed that the chemical and physical properties of graphene are crucially determined by their topological structures. Therefore, the atomically precise synthesis of graphene nanostructures is essential for studying their fundamental physiochemical properties as well as their introduction in promising applications. Among the large family of graphene nanostructures, those containing rich or fully zigzag‐edged structures exhibit unique electronic, magnetic, and optoelectronic properties owing to their spin‐polarized edge state. Prominent examples include the open‐shell biradical peri‐tetracene, π‐extended triangulene with triradicals, and fully zigzag‐edged graphene nanoribbons (GNRs) with localized edge states. Recent progress in the development of synthetic methodologies and strategies as well as characterization methods has rendered access to this class of unprecedented graphene nanostructures with rich zigzag edges, which used to be a purely molecular objective in theoretical chemistry. Thus, clear insight into the structure‐property relationships has become possible before exploring future applications in organic carbon‐based electronic and spintronic devices. In this minireview, we discuss the recent progress in the controlled synthesis of zigzag‐edged graphene nanostructures with different topologies through a bottom‐up synthetic strategy. |
Persistent Identifier | http://hdl.handle.net/10722/286162 |
ISSN | 2023 Impact Factor: 16.1 2023 SCImago Journal Rankings: 5.300 |
PubMed Central ID | |
ISI Accession Number ID |
DC Field | Value | Language |
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dc.contributor.author | Liu, J | - |
dc.contributor.author | Feng, X | - |
dc.date.accessioned | 2020-08-31T07:00:00Z | - |
dc.date.available | 2020-08-31T07:00:00Z | - |
dc.date.issued | 2020 | - |
dc.identifier.citation | Angewandte Chemie (International Edition), 2020, v. 59 n. 52, p. 23386-23401 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.uri | http://hdl.handle.net/10722/286162 | - |
dc.description.abstract | Both experimental and theoretical investigations have revealed that the chemical and physical properties of graphene are crucially determined by their topological structures. Therefore, the atomically precise synthesis of graphene nanostructures is essential for studying their fundamental physiochemical properties as well as their introduction in promising applications. Among the large family of graphene nanostructures, those containing rich or fully zigzag‐edged structures exhibit unique electronic, magnetic, and optoelectronic properties owing to their spin‐polarized edge state. Prominent examples include the open‐shell biradical peri‐tetracene, π‐extended triangulene with triradicals, and fully zigzag‐edged graphene nanoribbons (GNRs) with localized edge states. Recent progress in the development of synthetic methodologies and strategies as well as characterization methods has rendered access to this class of unprecedented graphene nanostructures with rich zigzag edges, which used to be a purely molecular objective in theoretical chemistry. Thus, clear insight into the structure‐property relationships has become possible before exploring future applications in organic carbon‐based electronic and spintronic devices. In this minireview, we discuss the recent progress in the controlled synthesis of zigzag‐edged graphene nanostructures with different topologies through a bottom‐up synthetic strategy. | - |
dc.language | eng | - |
dc.publisher | Wiley - VCH Verlag GmbH & Co. KGaA. The Journal's web site is located at http://www3.interscience.wiley.com/journal/26737/home | - |
dc.relation.ispartof | Angewandte Chemie (International Edition) | - |
dc.rights | This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License. | - |
dc.subject | Bottom-up synthesis | - |
dc.subject | Doping | - |
dc.subject | Graphene nanoribbons | - |
dc.subject | Magnetism | - |
dc.subject | Nanographenes | - |
dc.title | Synthetic Tailoring of Graphene Nanostructures with Zigzag‐Edged Topologies: Progress and Perspectives | - |
dc.type | Article | - |
dc.identifier.email | Liu, J: juliu@hku.hk | - |
dc.identifier.authority | Liu, J=rp02584 | - |
dc.description.nature | published_or_final_version | - |
dc.identifier.doi | 10.1002/anie.202008838 | - |
dc.identifier.pmid | 32720441 | - |
dc.identifier.pmcid | PMC7756885 | - |
dc.identifier.scopus | eid_2-s2.0-85092080900 | - |
dc.identifier.hkuros | 313176 | - |
dc.identifier.volume | 59 | - |
dc.identifier.issue | 52 | - |
dc.identifier.spage | 23386 | - |
dc.identifier.epage | 23401 | - |
dc.identifier.isi | WOS:000575230800001 | - |
dc.publisher.place | Germany | - |
dc.identifier.issnl | 1433-7851 | - |