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Article: Preparation of 1T′-Phase ReS 2 x Se 2(1- x) (x = 0-1) Nanodots for Highly Efficient Electrocatalytic Hydrogen Evolution Reaction

TitlePreparation of 1T′-Phase ReS <inf>2 x</inf> Se <inf>2(1- x)</inf> (x = 0-1) Nanodots for Highly Efficient Electrocatalytic Hydrogen Evolution Reaction
Authors
Issue Date2018
Citation
Journal of the American Chemical Society, 2018, v. 140, n. 27, p. 8563-8568 How to Cite?
AbstractAs a source of clean energy, a reliable hydrogen evolution reaction (HER) requires robust and highly efficient catalysts. Here, by combining chemical vapor transport and Li-intercalation, we have prepared a series of 1T′-phase ReS 2x Se 2(1-x) (x = 0-1) nanodots to achieve high-performance HER in acid medium. Among them, the 1T′-phase ReSSe nanodot exhibits the highest hydrogen evolution activity, with a Tafel slope of 50.1 mV dec -1 and a low overpotential of 84 mV at current density of 10 mA cm -2 . The excellent hydrogen evolution activity is attributed to the optimal hydrogen absorption energy of the active site induced by the asymmetric S vacancy in the highly asymmetric 1T′ crystal structure.
Persistent Identifierhttp://hdl.handle.net/10722/330009
ISSN
2023 Impact Factor: 14.4
2023 SCImago Journal Rankings: 5.489
ISI Accession Number ID

 

DC FieldValueLanguage
dc.contributor.authorLai, Zhuangchai-
dc.contributor.authorChaturvedi, Apoorva-
dc.contributor.authorWang, Yun-
dc.contributor.authorTran, Thu Ha-
dc.contributor.authorLiu, Xiaozhi-
dc.contributor.authorTan, Chaoliang-
dc.contributor.authorLuo, Zhimin-
dc.contributor.authorChen, Bo-
dc.contributor.authorHuang, Ying-
dc.contributor.authorNam, Gwang Hyeon-
dc.contributor.authorZhang, Zhicheng-
dc.contributor.authorChen, Ye-
dc.contributor.authorHu, Zhaoning-
dc.contributor.authorLi, Bing-
dc.contributor.authorXi, Shibo-
dc.contributor.authorZhang, Qinghua-
dc.contributor.authorZong, Yun-
dc.contributor.authorGu, Lin-
dc.contributor.authorKloc, Christian-
dc.contributor.authorDu, Yonghua-
dc.contributor.authorZhang, Hua-
dc.date.accessioned2023-08-09T03:37:09Z-
dc.date.available2023-08-09T03:37:09Z-
dc.date.issued2018-
dc.identifier.citationJournal of the American Chemical Society, 2018, v. 140, n. 27, p. 8563-8568-
dc.identifier.issn0002-7863-
dc.identifier.urihttp://hdl.handle.net/10722/330009-
dc.description.abstractAs a source of clean energy, a reliable hydrogen evolution reaction (HER) requires robust and highly efficient catalysts. Here, by combining chemical vapor transport and Li-intercalation, we have prepared a series of 1T′-phase ReS 2x Se 2(1-x) (x = 0-1) nanodots to achieve high-performance HER in acid medium. Among them, the 1T′-phase ReSSe nanodot exhibits the highest hydrogen evolution activity, with a Tafel slope of 50.1 mV dec -1 and a low overpotential of 84 mV at current density of 10 mA cm -2 . The excellent hydrogen evolution activity is attributed to the optimal hydrogen absorption energy of the active site induced by the asymmetric S vacancy in the highly asymmetric 1T′ crystal structure.-
dc.languageeng-
dc.relation.ispartofJournal of the American Chemical Society-
dc.titlePreparation of 1T′-Phase ReS <inf>2 x</inf> Se <inf>2(1- x)</inf> (x = 0-1) Nanodots for Highly Efficient Electrocatalytic Hydrogen Evolution Reaction-
dc.typeArticle-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1021/jacs.8b04513-
dc.identifier.pmid29870234-
dc.identifier.scopuseid_2-s2.0-85048215982-
dc.identifier.volume140-
dc.identifier.issue27-
dc.identifier.spage8563-
dc.identifier.epage8568-
dc.identifier.eissn1520-5126-
dc.identifier.isiWOS:000439009200031-

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